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NCHFNOIn the title compound, CHFNO, the pyridine ring is connected to a benzene ring by a -CH-NH- chain. The nitro group is twisted out of the pyridine ring plane [torsion angle O-N-C-C = 10.41 (10)°]. An intramolecular N-H⋯O hydrogen bond occurs. The fluorobenzene ring is disordered over two positions [occupancy ratio = 0.59 (3):0.41 (3)]. Intermolecular N-H⋯O and N-H⋯N hydrogen bonds stabilize the crystal structure.
Related literature
The title compound is an intermediate in the synthesis of analgesic drugs. For the analgesic properties of flupirtine (systematic name ethyl{2-amino-6-[(4-fluorobenzyl)amino]pyridin-3-yl}carbamate), see: Klawe & Maschke (2009 ▶). For synthetic procedures, see: Gerhard & Ilia (2010 ▶). For a related structure, see: Wang (2009 ▶).
Experimental
Crystal data
CHFNO
M
= 262.25
Monoclinic, inline-formula
a = 14.8187 (14) Å
b = 5.9972 (6) Å
c = 14.8840 (15) Å
β = 109.827 (1)°
V = 1244.3 (2) Å
Z = 4
Mo Kα radiation
μ = 0.11 mm
T = 298 K
0.38 × 0.15 × 0.11 mm
Data collection
Rigaku SCXmini CCD diffractometer
Absorption correction: multi-scan (CrystalClear; Rigaku, 2005 ▶) T
= 0.960, T
= 0.988
5923 measured reflections
2184 independent reflections
1169 reflections with I > 2σ(I)
R
= 0.056
Refinement
R[F
> 2σ(F
)] = 0.052
wR(F
) = 0.140
S = 1.03
2184 reflections
227 parameters
H-atom parameters constrained
Δρ = 0.21 e Å
Δρ = −0.22 e Å
Data collection: CrystalClear (Rigaku, 2005 ▶); cell refinement: CrystalClear; data reduction: CrystalClear; program(s) used to solve structure: SHELXS97 (Sheldrick, 2008 ▶); program(s) used to refine structure: SHELXL97 (Sheldrick, 2008 ▶); molecular graphics: ORTEP-3 for Windows (Farrugia, 1997 ▶) and PLATON (Spek, 2009 ▶); software used to prepare material for publication: SHELXL97.
Supplementary Material
Crystal structure: contains datablocks I, global. DOI: 10.1107/S1600536811018642/pv2411sup1.cif
Structure factors: contains datablocks I. DOI: 10.1107/S1600536811018642/pv2411Isup2.hkl
Supplementary material file. DOI: 10.1107/S1600536811018642/pv2411Isup3.cml
Additional supplementary materials: crystallographic information; 3D view; checkCIF report
Hydrogen-bond geometry (Å, °)
Symmetry codes: (i) inline-formula ; (ii) inline-formula .
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